Preparation of dimethoxyborane and analysis by Fourier transform infrared spectroscopy

Andreas Bernas, Birgitta Peltopakka, Päivi Mäki-Arvela, Kari Eränen, Tapio Salmi, Dmitry Yu. Murzin*

*Corresponding author for this work

Research output: Contribution to journalArticleScientificpeer-review

3 Citations (Scopus)

Abstract

Dimethoxyborane was prepared by the reaction of trimethoxyboroxine, sodium borohydride and trimethyl borate in diethylene glycol dimethyl ether solvent at 70°C under atmospheric pressure followed by distillation to increase the purity and analyzed in liquid phase by FT-IR. The concentration of dimethoxyborane was identified by hydrolysis with water, which yields boric acid, methanol and hydrogen, whereas the generated hydrogen was analyzed by the mass detector of a volumetric flow apparatus. The FT-IR absorbance peak area showed a linear dependence on dimethoxyborane concentration in the wavenumber range 873 to 950 cm-1 for samples with dimethoxyborane concentrations 0 to 6.2 wt% in trimethyl borate. Data fitting using the least square method gave an R 2 value of 97%.

Original languageEnglish
Pages (from-to)645-654
Number of pages10
JournalResearch on Chemical Intermediates
Volume33
Issue number7
DOIs
Publication statusPublished - 2007
MoE publication typeA1 Journal article-refereed

Funding

This work is part of the activities at the Åbo Akademi Process Chemistry Centre within the Finnish Centre of Excellence Programme (2000–2011) by the Academy of Finland. Financial support from Finnish Chemicals Oy is gratefully acknowledged.

Keywords

  • Dimethoxyborane
  • FT-IR
  • Hydrolysis
  • Trimethylborate

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