Physical Modelling of Large-Area Single-Molecule Organic Transistors

Fabrizio Torricelli; Eleonora MacChia; Paolo Bollella; Cinzia Di Franco; Zsolt M. Kovacs-Vajna; Gaetano Scamarcio; Luisa Torsi

doi:10.1109/FLEPS53764.2022.9781507

Physical Modelling of Large-Area Single-Molecule Organic Transistors

Fabrizio Torricelli^*, Eleonora MacChia, Paolo Bollella, Cinzia Di Franco, Zsolt M. Kovacs-Vajna, Gaetano Scamarcio, Luisa Torsi

^*Corresponding author for this work

Physics

Research output: Chapter in Book/Conference proceeding › Published conference proceeding › Scientific › peer-review

Abstract

Single-Molecule organic transistors embedding a large-area bioreceptor surface can potentially revolutionize the current medical diagnostic approaches. For instance, sensing a single molecule in a biological fluid can provide early and noninvasive detection of a disease. The development of a reliable and multiplexed electronic large-area single-molecule technology urgently requires the improvement of our current understanding. Here we propose a physical model of large-area single-molecule organic transistor sensors. The model describes the electrical measurements and provides meaningful information about the sensor operation. The bioelectronic responses can be linked to the physical parameters and guidelines for device optimization are suggested.

Original language	English
Title of host publication	2022 IEEE International Conference on Flexible and Printable Sensors and Systems (FLEPS)
Publisher	the Institute of Electrical and Electronics Engineers, Inc.
ISBN (Electronic)	9781665442732
DOIs	https://doi.org/10.1109/FLEPS53764.2022.9781507
Publication status	Published - 2022
MoE publication type	A4 Article in a conference publication
Event	2022 IEEE International Conference on Flexible and Printable Sensors and Systems, FLEPS 2022 - Vienna, Austria Duration: 10 Jul 2022 → 13 Jul 2022

Publication series

Name	FLEPS 2022 - IEEE International Conference on Flexible and Printable Sensors and Systems, Proceedings

Conference

Conference	2022 IEEE International Conference on Flexible and Printable Sensors and Systems, FLEPS 2022
Country/Territory	Austria
City	Vienna
Period	10/07/22 → 13/07/22

Funding

As displayed in the inset of Fig. 3b, is close to zero when there are no ligands in the analyte solution, it strongly increases after incubating the gate into analyte containing few molecules, it further increases when the gate is incubated at The authors would like to acknowledge the financial support of the European Commission for the projects SiMBiT (Horizon 2020 ICT, contract n°824946).

Keywords

bio-sensor
modelling
organic transistor
single-molecule

Access to Document

10.1109/FLEPS53764.2022.9781507

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Torricelli, F., MacChia, E., Bollella, P., Di Franco, C., Kovacs-Vajna, Z. M., Scamarcio, G., & Torsi, L. (2022). Physical Modelling of Large-Area Single-Molecule Organic Transistors. In 2022 IEEE International Conference on Flexible and Printable Sensors and Systems (FLEPS) (FLEPS 2022 - IEEE International Conference on Flexible and Printable Sensors and Systems, Proceedings). the Institute of Electrical and Electronics Engineers, Inc.. https://doi.org/10.1109/FLEPS53764.2022.9781507

Torricelli, Fabrizio ; MacChia, Eleonora ; Bollella, Paolo et al. / Physical Modelling of Large-Area Single-Molecule Organic Transistors. 2022 IEEE International Conference on Flexible and Printable Sensors and Systems (FLEPS). the Institute of Electrical and Electronics Engineers, Inc., 2022. (FLEPS 2022 - IEEE International Conference on Flexible and Printable Sensors and Systems, Proceedings).

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abstract = "Single-Molecule organic transistors embedding a large-area bioreceptor surface can potentially revolutionize the current medical diagnostic approaches. For instance, sensing a single molecule in a biological fluid can provide early and noninvasive detection of a disease. The development of a reliable and multiplexed electronic large-area single-molecule technology urgently requires the improvement of our current understanding. Here we propose a physical model of large-area single-molecule organic transistor sensors. The model describes the electrical measurements and provides meaningful information about the sensor operation. The bioelectronic responses can be linked to the physical parameters and guidelines for device optimization are suggested.",

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author = "Fabrizio Torricelli and Eleonora MacChia and Paolo Bollella and \{Di Franco\}, Cinzia and Kovacs-Vajna, \{Zsolt M.\} and Gaetano Scamarcio and Luisa Torsi",

note = "BOF 15/1 EK Funding Information: As displayed in the inset of Fig. 3b, is close to zero when there are no ligands in the analyte solution, it strongly increases after incubating the gate into analyte containing few molecules, it further increases when the gate is incubated at The authors would like to acknowledge the financial support of the European Commission for the projects SiMBiT (Horizon 2020 ICT, contract n°824946). Publisher Copyright: {\textcopyright} 2022 IEEE.; 2022 IEEE International Conference on Flexible and Printable Sensors and Systems, FLEPS 2022 ; Conference date: 10-07-2022 Through 13-07-2022",

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doi = "10.1109/FLEPS53764.2022.9781507",

language = "English",

series = "FLEPS 2022 - IEEE International Conference on Flexible and Printable Sensors and Systems, Proceedings",

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Torricelli, F, MacChia, E, Bollella, P, Di Franco, C, Kovacs-Vajna, ZM, Scamarcio, G & Torsi, L 2022, Physical Modelling of Large-Area Single-Molecule Organic Transistors. in 2022 IEEE International Conference on Flexible and Printable Sensors and Systems (FLEPS). FLEPS 2022 - IEEE International Conference on Flexible and Printable Sensors and Systems, Proceedings, the Institute of Electrical and Electronics Engineers, Inc., 2022 IEEE International Conference on Flexible and Printable Sensors and Systems, FLEPS 2022, Vienna, Austria, 10/07/22. https://doi.org/10.1109/FLEPS53764.2022.9781507

Physical Modelling of Large-Area Single-Molecule Organic Transistors. / Torricelli, Fabrizio; MacChia, Eleonora; Bollella, Paolo et al.
2022 IEEE International Conference on Flexible and Printable Sensors and Systems (FLEPS). the Institute of Electrical and Electronics Engineers, Inc., 2022. (FLEPS 2022 - IEEE International Conference on Flexible and Printable Sensors and Systems, Proceedings).

Research output: Chapter in Book/Conference proceeding › Published conference proceeding › Scientific › peer-review

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AU - MacChia, Eleonora

AU - Bollella, Paolo

AU - Di Franco, Cinzia

AU - Kovacs-Vajna, Zsolt M.

AU - Scamarcio, Gaetano

AU - Torsi, Luisa

N1 - BOF 15/1 EK Funding Information: As displayed in the inset of Fig. 3b, is close to zero when there are no ligands in the analyte solution, it strongly increases after incubating the gate into analyte containing few molecules, it further increases when the gate is incubated at The authors would like to acknowledge the financial support of the European Commission for the projects SiMBiT (Horizon 2020 ICT, contract n°824946). Publisher Copyright: © 2022 IEEE.

PY - 2022

Y1 - 2022

N2 - Single-Molecule organic transistors embedding a large-area bioreceptor surface can potentially revolutionize the current medical diagnostic approaches. For instance, sensing a single molecule in a biological fluid can provide early and noninvasive detection of a disease. The development of a reliable and multiplexed electronic large-area single-molecule technology urgently requires the improvement of our current understanding. Here we propose a physical model of large-area single-molecule organic transistor sensors. The model describes the electrical measurements and provides meaningful information about the sensor operation. The bioelectronic responses can be linked to the physical parameters and guidelines for device optimization are suggested.

AB - Single-Molecule organic transistors embedding a large-area bioreceptor surface can potentially revolutionize the current medical diagnostic approaches. For instance, sensing a single molecule in a biological fluid can provide early and noninvasive detection of a disease. The development of a reliable and multiplexed electronic large-area single-molecule technology urgently requires the improvement of our current understanding. Here we propose a physical model of large-area single-molecule organic transistor sensors. The model describes the electrical measurements and provides meaningful information about the sensor operation. The bioelectronic responses can be linked to the physical parameters and guidelines for device optimization are suggested.

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KW - modelling

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KW - single-molecule

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BT - 2022 IEEE International Conference on Flexible and Printable Sensors and Systems (FLEPS)

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ER -

Torricelli F, MacChia E, Bollella P, Di Franco C, Kovacs-Vajna ZM, Scamarcio G et al. Physical Modelling of Large-Area Single-Molecule Organic Transistors. In 2022 IEEE International Conference on Flexible and Printable Sensors and Systems (FLEPS). the Institute of Electrical and Electronics Engineers, Inc. 2022. (FLEPS 2022 - IEEE International Conference on Flexible and Printable Sensors and Systems, Proceedings). doi: 10.1109/FLEPS53764.2022.9781507

Physical Modelling of Large-Area Single-Molecule Organic Transistors

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